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• W4224287193 abstract "A simple and low-cost tandem sulfonylation/cyclization of 1,5-diene, aryldiazonium salt, and DABCO·(SO2)2 is disclosed. This base-promoted multicomponent reaction can provide a green and economic synthesis of sulfonylated pyrrolidones under transition-metal-free and moisture/oxygen-insensitive reaction conditions, thus delivering a wide range of sulfonylated pyrrolidones in moderate to high yields with excellent functional group compatibility. A plausible mechanism involving a radical process is proposed, which demonstrates highly chemoselective trapping of the aryl radical with SO2 species, and a regioselective sulfonylation/cyclization protocol in this reaction." @default.
• W4224287193 created "2022-04-26" @default.
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• W4224287193 date "2022-04-19" @default.
• W4224287193 modified "2023-09-29" @default.
• W4224287193 title "Regioselective Radical-Relay Sulfonylation/Cyclization Protocol to Sulfonylated Pyrrolidones under Transition-Metal-Free Conditions" @default.
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• W4224287193 doi "https://doi.org/10.1021/acs.joc.2c00381" @default.
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