Matches in SemOpenAlex for { <https://semopenalex.org/work/W4224678416> ?p ?o ?g. }
- W4224678416 abstract "Abstract A new zinc‐based metal‐organic framework (MOF) Zn 2 (OAB) [OAB 4− =4,4′‐(oxalylbis(azanediyl))bis(2‐oxidobenzoate)), analogous to a well‐studied MOF‐74 structure, was solvothermal synthesized and characterized. The Zn 2 (OAB) frameworks exhibited accessible mesopore channels (24 Å) and high porosity (S BET =3115 m 2 g −1 ). The presence of the high density of both Lewis acidic Zn sites and −NH− groups derived from the organic OAB 4− unit make Zn 2 (OAB) a promising candidate for catalysis Paal‐Knorr N ‐substituted pyrroles synthesis. As such, Zn 2 (OAB) exhibited excellent catalytic activity in the synthesis of 2,5‐dimethyl‐1‐phenyl‐1 H ‐pyrrole with a yield of 96 % at 70 °C for 16 min. Notably, the catalytic activity of Zn 2 (OAB) outperformed that of homogeneous, heterogeneous catalysts, and representative Zn‐based MOFs (ZIF‐8, MOF‐5, Zn‐MOF‐74). The Zn 2 (OAB) was also demonstrated to be reused up to eight times without noteworthy loss of its activity." @default.
- W4224678416 created "2022-04-27" @default.
- W4224678416 creator A5061522035 @default.
- W4224678416 creator A5086899571 @default.
- W4224678416 date "2022-04-25" @default.
- W4224678416 modified "2023-10-14" @default.
- W4224678416 title "A New Zinc‐Based Metal‐Organic Framework for Catalytic Synthesis of <i>N</i>‐Substituted Pyrroles" @default.
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- W4224678416 doi "https://doi.org/10.1002/slct.202200592" @default.
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