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- W4224723114 abstract "Photocatalytic synthesis has emerged as an efficient route to transform CO2 into functionalized organic carbamates by photocatalysis. Herein, a catalyst-free carbamoyloxylation of arylacetones with CO2 and amines under visible light was developed for the synthesis of O-β-oxoalkyl carbamates in yields up to 93%. This protocol proceeded smoothly with the assistance of inexpensive carbon tetrabromide at room temperature under atmospheric CO2 pressure, leading to simultaneous construction of C-O and C-N bonds. Mechanism studies suggested the photoinduced hydrogen atom transfer (HAT) pathway followed by radical addition or single electron transfer (SET)." @default.
- W4224723114 created "2022-04-27" @default.
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- W4224723114 date "2022-01-01" @default.
- W4224723114 modified "2023-10-17" @default.
- W4224723114 title "Visible light-driven carbamoyloxylation of the α-C(sp<sup>3</sup>)–H bond of arylacetones <i>via</i> radical-initiated hydrogen atom transfer" @default.
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- W4224723114 doi "https://doi.org/10.1039/d2cc01761j" @default.
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