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- W4224879953 abstract "The feasibility of laser cooling of AuF molecule and its cation are investigated from vibrational and rotational perspectives. The spectroscopy of AuF molecule and AuF+ molecular cation are obtained by the method of multireference configuration interaction plus Davidson correction (MRCI + Q) and spin-orbit coupling (SOC) effect. On account of the accurate molecular spectroscopy and the transition dipole moment, the Franck-Condon factors and radiative lifetimes of AuF molecule and AuF+ molecular cation are calculated. Comparing the criterias of laser cooling candidate molecules, the AuF is an excellent candidate for laser cooling and while AuF+ is not sutable. The b3Π0+ ↔ Χ1Σ+0+ transition of AuF is selected for laser cooling and an optical cycling scheme is proposed. The scheme possesses highly diagonally Franck-Condon factors and the scattered photons achieve ∼ 104. Furthermore, the rotational transition analysis is also included in our work and found that its Franck Condon factors and Einstein coefficients are undistorted. Our work could provide theoretical support and accelerate the laser cooling of AuF molecules in experiments." @default.
- W4224879953 created "2022-04-27" @default.
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- W4224879953 date "2022-09-01" @default.
- W4224879953 modified "2023-10-01" @default.
- W4224879953 title "Spectroscopy and rovibrational cooling of AuF and its cation" @default.
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- W4224879953 doi "https://doi.org/10.1016/j.saa.2022.121279" @default.
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