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- W4224936680 abstract "Described herein is a highly enantioselective route to β-quaternary δ-lactams by palladium/pyridine-dihydroisoquinoline (PyDHIQ)-catalyzed conjugate arylations. Notably, the effect of π-interactions on the high enantioselectivity was elucidated by DFT calculations and noncovalent interaction (NCI) analysis. The skeleton of the PyDHIQ ligand plays a key role in the formation of attractive noncovalent interactions with substrates in an enantioselectivity-determining step. The developed methodology was successfully applied to the asymmetric formal synthesis of (−)-picenadol." @default.
- W4224936680 created "2022-04-28" @default.
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- W4224936680 date "2022-04-27" @default.
- W4224936680 modified "2023-10-02" @default.
- W4224936680 title "Palladium Catalysis Featuring Attractive Noncovalent Interactions Enabled Highly Enantioselective Access to β-Quaternary δ-Lactams" @default.
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- W4224936680 doi "https://doi.org/10.1021/acscatal.2c00541" @default.
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