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- W4224981503 abstract "Abstract One-photon-absorbing photosensitizers are commonly used in homogeneous photocatalysis which require the absorption of ultraviolet (UV) /visible light to populate the desired excited states with adequate energy and lifetime. Nevertheless, the limited penetration depth and competing absorption by organic substrates of UV/visible light calls upon exploring the utilization of longer-wavelength irradiation, such as near-infrared light (λ irr > 700 nm). Despite being found applications in photodynamic therapy and bioimaging, two-photon absorption (TPA), the simultaneous absorption of two photons by one molecule, has been rarely explored in homogeneous photocatalysis. Herein, we report a group of ruthenium polypyridyl complexes possessing TPA capability that can drive a variety of organic transformations upon irradiation with 740 nm light. We demonstrate that these TPA ruthenium complexes can operate in an analogous manner as one-photon-absorbing photosensitizers for both energy-transfer and photoredox reactions, as well as function in concert with a transition metal co-catalyst for metallaphotoredox C–C coupling reactions." @default.
- W4224981503 created "2022-04-28" @default.
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- W4224981503 date "2022-04-28" @default.
- W4224981503 modified "2023-10-14" @default.
- W4224981503 title "Two-photon-absorbing ruthenium complexes enable near infrared light-driven photocatalysis" @default.
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- W4224981503 doi "https://doi.org/10.1038/s41467-022-29981-3" @default.
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