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• W4225105076 abstract "The selective adsorption mechanisms involved in the competitive adsorption of five iodinated trihalomethanes (I-THMs) onto dithiolglycol and (3-mercaptopropyl)-trimethoxy functionalized HKUST-1 (HK-SH and HK-MPTS, respectively) were investigated by single- and mixed-batch adsorption. HK-SH had the highest adsorption rates and capacities for the five I-THMs, followed by HK-MPTS and pristine HKUST-1, even though the porosity and surface area decreased after modification. The primary adsorptive mechanism of HK-SH consists of ion-dipole interactions of I-THMs with the protonated hydroxyl and thiol groups at the metal (Cu) node, which is supported by Lewis acid-base reactions via Cu-Cu complex and π-π interactions. In a mixed solute, bromodiiodomethane, which was the most hydrophobic and had the smallest molecular size, exhibited the most competitive adsorption on HK-SH. In contrast, the selective adsorption of I-THMs onto HK-MPTS was affected by their log Kow values, causing hydrophobic partitioning onto the alkyl chain of the mercaptopropyl group. Iodinated haloforms tend to achieve a higher adsorption rate and capacity than chlorinated and brominated haloforms via hydrophobic partitioning. Moreover, dithiolglycol grafted onto HK-SH can better promote the excellent selective adsorption performance of iodoacetamide than dichloroiodomethane and iodoacetic acid in both single- and mixed-solute solutions due to hydrogen bonding via the -NH2 group of diiodoacetamide." @default.
• W4225105076 created "2022-04-30" @default.
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• W4225105076 date "2022-08-01" @default.
• W4225105076 modified "2023-09-25" @default.
• W4225105076 title "Selective adsorption mechanisms of iodinated trihalomethanes onto thiol-functionalized HKUST-1s in a mixed solute" @default.
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• W4225105076 doi "https://doi.org/10.1016/j.jenvman.2022.115099" @default.
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