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• W4225108114 abstract "Photocatalytic CO2 reduction is one of the most cost-effective and environmentally friendly techniques of converting CO2 into high-value compounds and/or fuels. However, the performance of most current photocatalytic CO2 reduction catalysts is less than satisfactory for practical applications. Here, we synthesized a heterogeneous structure by integrating Cu2O and a porphyrin hydrogen-bonded organic framework (PFC-45), which was then fabricated into a thin-film catalyst on carbolic paper (CP) using a facile electrophoretic deposition technology. With improved electron-hole separation efficiency and visible-light-harvesting ability, this film (PFC-45/Cu2O@CP) significantly enhanced CO2-to-CO photoreduction, exceeding 2.4 and 3.2 times that of PFC-45@CP and PFC-45/Cu2O particles, respectively. Remarkably, PFC-45/Cu2O@CP also exhibited high selectivity (99%) and outstanding activity (11.81 μmol g-1 h-1) for photocatalytic CO2 reduction in pure water without any sacrificial agent. This work demonstrates a new strategy to design photocatalysts for efficient CO2 reduction." @default.
• W4225108114 created "2022-04-30" @default.
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• W4225108114 date "2022-04-27" @default.
• W4225108114 modified "2023-10-16" @default.
• W4225108114 title "Facile Preparation of Hydrogen-Bonded Organic Framework/Cu₂O Heterostructure Films via Electrophoretic Deposition for Efficient CO₂ Photoreduction" @default.
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• W4225108114 doi "https://doi.org/10.1021/acsami.2c02917" @default.
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