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- W4225264216 endingPage "155640" @default.
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- W4225264216 abstract "In electrocatalytic reduction of nitrates to nitrogen, key issues are electrode activity, sustainable materials, preparation methods and cost. Herein, lignin, Fe3+ ion, and non-ionic surfactant were combined with evaporation-induced self-assembly (EISA) to prepare zero-valent Fe-dispersed ordered mesoporous carbon (OMC) electrode materials denoted as Fe#OMC. The method developed for preparing Fe-coordinated OMC material avoids the use of toxic phenols, aldehyde reagents and metal doping compounds. When synthesized Fe#OMC samples were applied as electrode materials for the electrocatalytic reduction of nitrate in aqueous solutions, maximum nitrate nitrogen removal was as high as 5373 mg N·g-1 Fe from aqueous solutions containing 400 mg·L-1 NO3--N, while nitrogen selectivity was close to 100%, exceeding catalytic performance of comparable materials. Active hydrogen produced by electrolysis of water during the reaction re-reduced Fe ions formed in the OMC material and stabilized Fe#OMC electrode performance and recycle. The Fe#OMC electrode is self-renewing with respect to its Fe zero-valent state, is simple to prepare from sustainable materials and is effective for electrocatalytic reduction of nitrate or nitrogen-containing compounds in water." @default.
- W4225264216 created "2022-05-04" @default.
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- W4225264216 date "2022-08-01" @default.
- W4225264216 modified "2023-10-14" @default.
- W4225264216 title "Synthesis of self-renewing Fe(0)-dispersed ordered mesoporous carbon for electrocatalytic reduction of nitrates to nitrogen" @default.
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- W4225264216 doi "https://doi.org/10.1016/j.scitotenv.2022.155640" @default.
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