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- W4225270680 abstract "Non-covalent interactions play an essential role in the folding and self-assembly of large biological assemblies. These interactions are not only a driving force for the formation of large structures but also control conformation and com-plementary shapes of subcomponents that promote the diversity of structures and functions of the resulting assemblies. Understanding how non-covalent interactions direct self-assembly and the effect of conformation and complementary shapes on self-assembled structures will help design artificial supramolecular systems with extended components and functions. Herein, we develop a strategy for controlling more complex self-assembly with lower symmetry and flexible building blocks that combine endohedral non-covalent interactions with a dual curvature in the ligand backbone to give additional shape complementarity. A Diels-Alder reaction was used to break the symmetry of the diazaanthracene units of the ligands to give dual curvature ligands with different shapes and endohedral groups (L1-L3). The self-assembly studies of these ligands demonstrated that non-covalent interactions and shape complementary effectively control the self-assembly and enable the design of cages for supramolecular catalysis." @default.
- W4225270680 created "2022-05-04" @default.
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- W4225270680 date "2022-05-02" @default.
- W4225270680 modified "2023-09-27" @default.
- W4225270680 title "Design of catalytic metal-organic assemblies via shape complementarity and conformational constraints in dual curvature ligands" @default.
- W4225270680 doi "https://doi.org/10.26434/chemrxiv-2021-4z45w-v2" @default.
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