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- W4225281719 endingPage "2200122" @default.
- W4225281719 startingPage "2200122" @default.
- W4225281719 abstract "High-performance lithium-ion batteries (LIBs) are required for the rising energy storage demand, while their development depends mainly on cathode materials. Vanadium-based compounds are considered to be promising due to the feasibility of multielectron reactions arising from the rich valence states of vanadium (+2 to +5). Herein, for the first time the electrochemical properties of a vanadium-based fluoroxide, β-KVOF3, as a cathode for LIBs, are reported. After optimization, a reversible capacity as high as 274 mAh g−1, a stable 300 cycles lifetime, and an energy density comparable to LiFePO4 (650 vs 550 Wh kg−1) are achieved. Experiments and simulation study of reaction mechanism illustrate that such performance originates from the reversible V3+/V5+ redox reaction, high structural stability of β-KVOF3, and the pseudocapacitive process during charging and discharging. This study reveals that β-KVOF3 is a promising cathode for Li-ion storage and provides a new design idea for developing high-performance LIBs cathode materials." @default.
- W4225281719 created "2022-05-04" @default.
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- W4225281719 date "2022-05-01" @default.
- W4225281719 modified "2023-10-14" @default.
- W4225281719 title "A Vanadium‐Based Fluoroxide Cathode Material for Lithium‐Ion Storage with High Energy Density" @default.
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- W4225281719 doi "https://doi.org/10.1002/adsu.202200122" @default.
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