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• W4225384813 endingPage "276" @default.
• W4225384813 startingPage "241" @default.
• W4225384813 abstract "ABSTRACT Extensional deformations represent an effective stimulus to explore the rich rheological response of branched polymers and elastomers, enabling the design of polymers with specific molecular structure. However, probing the polymer behavior at large deformations is often limited by the experimental devices. We here present an alternative use of the Sentmanat Extensional Rheometer (SER) that allows Hencky strain units much larger than the maximum value achievable, ∼3.6. The proposed procedure consists of an oblique positioning of the sample in the measuring area. If a small inclination of the sample is used, the departure from the ideal uniaxial flow is negligible at Hencky strains &lt;1, and nearly zero for larger values. Experimental results in the linear viscoelastic regime are compared with the double reptation model in order to discern polydispersity and branching effects, whereas the extensional rheology data are contrasted with the molecular stress function theory (MSF), revealing important information about the polymer structure, especially on the long-chain branching (LCB). Finally, the analysis of sample failure upon elongation allowed us to correlate the polymer structure to the rheological behavior during mixing processes." @default.
• W4225384813 created "2022-05-05" @default.
• W4225384813 creator A5002155424 @default.
• W4225384813 creator A5025611217 @default.
• W4225384813 creator A5063333028 @default.
• W4225384813 creator A5070723386 @default.
• W4225384813 creator A5088450032 @default.
• W4225384813 creator A5088775567 @default.
• W4225384813 date "2022-04-01" @default.
• W4225384813 modified "2023-10-12" @default.
• W4225384813 title "ALTERNATIVE USE OF THE SENTMANAT EXTENSIONAL RHEOMETER TO INVESTIGATE THE RHEOLOGICAL BEHAVIOR OF INDUSTRIAL RUBBERS AT VERY LARGE DEFORMATIONS" @default.
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