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• W4225413949 startingPage "056512" @default.
• W4225413949 abstract "Nowadays, to relieve the environmental issues and the energy depletion, one of the most practicable and feasible technologies is the electrochemical reduction of CO 2 to high value added chemicals. In this aspect, the bottleneck is to develop novel catalysts with high efficiency and selectivity. Based on this idea, in this work, a series of two dimensional transitional metal doped trihydroxytriaminophenalenyl, i.e., M 3 (THTAP) 2 , have been studied as the catalysts for CO 2 reduction reaction (CO 2 RR). Our study showed that these catalysts are stable and have metallic character, which is conducive to electroreduction reaction. Products CH 4 , CH 3 OH and HCOOH are obtained for the studied catalysts. Cr 3 (THTAP) 2 is the best catalyst for producing CH 4 . Ir 3 (THTAP) 2 produces CH 3 OH as the final product and the overpotential is 0.34 V. Both Pt 3 (THTAP) 2 and Pd 3 (THTAP) 2 are good CO 2 RR catalysts to produce HCOOH with the small overpotentials of 0.17 and 0.23 V, respectively. Thus, these two dimensional transition metal organic frameworks exhibit great potential as the electrochemical catalysts for high performance CO 2 electro-catalytic process. We anticipate that this work may shed new light on the development of high performance metal organic framework based electrocatalysts." @default.
• W4225413949 created "2022-05-05" @default.
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• W4225413949 date "2022-05-01" @default.
• W4225413949 modified "2023-10-14" @default.
• W4225413949 title "Theoretical Insights on the Two-Dimensional Transitional Metal Trihydroxytriaminophenalenyl for Highly Efficient Carbon Dioxide Electroreduction" @default.
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• W4225413949 doi "https://doi.org/10.1149/1945-7111/ac6c52" @default.
• W4225413949 hasPublicationYear "2022" @default.
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