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• W4225510372 abstract "Reasonable design of the structure and complementary compounding of electrode materials is helpful to enhance capacitive deionization (CDI) performance. Herein, a novel 0D-3D hierarchical electrode material containing Na2Ti3O7 nanoparticles anchored at hollow red blood cell (HRBC)-like nitrogen-rich carbon (HRBC-NTO/N-C-60) was prepared via selective protection, pyrolysis, and alkalization. Specifically, a HRBC-like NH2-MIL-125-based material (HRBC-MOF-60) was first constructed by a selective protection approach of tannic acid (TN), which addresses the shortcomings of using sacrificial templates or corrosive agents. Afterwards, HRBC-NTO/N-C-60 was obtained in situ by annealing and alkalization of HRBC-MOF-60. The nitrogen-rich carbon with a HRBC-like structure has the ability to rapidly transport electrons, and its porous structure enables remarkable charge transfer. Benefiting from the grafted 3D N-doped porous carbon with a HRBC-like structure, well-dispersed 0D Na2Ti3O7 nanoparticles, and satisfactory bonding effects, HRBC-NTO/N-C-60 exhibited high specific capacitance and fast ionic and electronic diffusion kinetics. Moreover, HRBC-NTO/N-C-60 was well-suited for desalination by functioning as a cathode material for capacitive deionization (CDI), and delivering a high desalination capacity of 66.8 mg g-1 in 200 mg L-1 NaCl solution at 1.4 V. This work introduces an excellent high-performance candidate for electrochemical deionization as well as affording afflatus for accurately inventing OD-3D hierarchical materials with hollow structures." @default.
• W4225510372 created "2022-05-05" @default.
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• W4225510372 date "2022-01-01" @default.
• W4225510372 modified "2023-10-14" @default.
• W4225510372 title "<i>In situ</i> anchor of Na₂Ti₃O₇ in nitrogen-rich carbon hollow red blood cell-like structure as a 0D-3D hierarchical electrode material for efficient electrochemical desalination" @default.
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• W4225510372 doi "https://doi.org/10.1039/d1sc06476b" @default.
• W4225510372 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/35656142" @default.
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