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• W4225607546 startingPage "08LT01" @default.
• W4225607546 abstract "The discovery of group IV and V elemental xene's with topologically non-trivial characters in their honeycomb lattice structure (HLS) has led to extensive efforts in realising analogous behaviour in group VI elemental monolayers. Theoretically; it was concluded that, group VI elemental monolayers cannot exist in HLS. However, some recent experimental evidence suggests that group VI elemental monolayers can be realised in HLS. In this letter, we report HLS of group VI elemental monolayer (such as, tellurene) can be realised to be dynamically stable when functionzalised with oxygen. The functionalization leads to, peculiar orbital filtering effects and broken spatial inversion symmetry which gives rise to the non-trivial topological character. The exotic quantum behaviour of this system is characterized by, spin-orbit coupling induced large-gap (≈0.36 eV) with isolated Dirac cone along the edges indicating potential room temperature spin-transport applications. Further investigations of spin Hall conductivity and the Berry curvatures unravel high conductivity as compared to previously explored xene's alongside the potential valley Hall effects. The non-trivial topological character is quantified in terms of theZ2invariant asν= 1 and Chern numberC= 1. Also, for practical purposes, we report that,hBN/TeO/hBN quantum-wells can be strain engineered to realize a sizeable non-trivial gap (≈0.11 eV). We finally conclude that, functionalization of group VI elemental monolayer with oxygen gives rise to, exotic quantum properties which are robust against surface oxidation and degradations while providing viable electronic degrees of freedom for spintronic/valleytronic applications." @default.
• W4225607546 created "2022-05-05" @default.
• W4225607546 creator A5009902080 @default.
• W4225607546 creator A5012361511 @default.
• W4225607546 date "2021-11-30" @default.
• W4225607546 modified "2023-09-26" @default.
• W4225607546 title "Functionalized tellurene; a candidate large-gap 2D topological insulator" @default.
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• W4225607546 doi "https://doi.org/10.1088/1361-648x/ac3a47" @default.
• W4225607546 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/34787102" @default.
• W4225607546 hasPublicationYear "2021" @default.
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