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• W4225761614 endingPage "103546" @default.
• W4225761614 startingPage "103546" @default.
• W4225761614 abstract "• Bi 2 MoO 6 / MIL-101 (Fe) as novel catalyst was synthesized via the solvothermal procedure. • Effect of water matrix was explored on pollutant removal efficiency. • Charge transfer mechanism for Bi 2 MoO 6 / MIL-101 (Fe) was investigated. • The impact of process factors in contaminant removal efficiency were evaluated by using CCF. The integration of Bi 2 MoO 6 with MIL-101(Fe) as a novel structure enhanced photocatalytic activity for RhB degradation. Bi 2 MoO 6 /MIL-101(Fe) composites were synthesized via the solvothermal procedure and characterized by XRD, EDX, FE-SEM, TEM, FT-IR, BET, TGA, UV–vis DRS, and PL. The optimal molar ratio Bi 2 MoO 6 :MIL-101(Fe) equal to 1:1 showed better photocatalytic activity than Bi 2 MoO 6 and MIL-101(Fe) and other heterostructure composites. The effect of pH (5–9), reaction time (60–120 min), catalyst concentration (0.1–0.5 g/L), and dye concentration (10–20 ppm) were investigated on the removal performance of RhB by using central composite face-centered (CCF). In the optimal process factors where the [Catalyst]:0.4 g/L, [RhB]:20 ppm, pH: 6.5, irradiation time: 120 min, the RhB and TOC removal efficiency were 85% and 84.2%, respectively. The holes and superoxide radicals played a major role in the degradation of RhB. The addition of salt (NaCl, Na 2 SO 4 , and NaHCO 3 ) at different concentrations (100, 200, 400, and 800 ppm) revealed that the salts have an inhibitory role in the photocatalytic performance. At low concentrations of 100 ppm, the salts had a negative effect on removal efficiency (k Pure water = 0.0155 min −1 , k NaCl = 0.0075 min −1 , k Na2SO4 = 0.0132 min −1 , k NaHCO3 = 0.006 min −1 ). Increasing the salt concentration to 800 ppm caused improved efficiency for NaCl (k NaCl = 0.0141 min −1 ), while for Na 2 SO 4 this trend was decreasing (k Na2SO4 = 0.011 min −1 ), and for NaHCO 3 sharply diminished (k NaHCO3 = 0.0026 min −1 )." @default.
• W4225761614 created "2022-05-05" @default.
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• W4225761614 date "2022-05-01" @default.
• W4225761614 modified "2023-10-06" @default.
• W4225761614 title "Synthesis and characterization of Bi2MoO6/MIL-101(Fe) as a novel composite with enhanced photocatalytic performance: Effect of water matrix and reaction mechanism" @default.
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• W4225761614 doi "https://doi.org/10.1016/j.apt.2022.103546" @default.
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