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• W4226031763 abstract "Lithium‐ion batteries are commonly used for electrical energy storage in portable devices and are promising systems for large‐scale energy storage. However, their application is still limited due to electrode degradation and stability issues. To enhance the fundamental understanding of electrode degradation, we report on the Raman spectroscopic characterization of LiCoO 2 cathode materials of working Li‐ion batteries. To facilitate the spectroscopic analysis of the solid electrolyte interface (SEI), we apply in situ surface‐enhanced Raman spectroscopy under battery working conditions by using Au nanoparticles coated with a thin SiO 2 layer (Au@SiO 2 ). We observe a surface‐enhanced Raman signal of Li 2 CO 3 at 1090 cm −1 during electrochemical cycling as an intermediate. Its formation/decomposition highlights the role of Li 2 CO 3 as a component of the SEI on LiCoO 2 composite cathodes. Our results demonstrate the potential of Raman spectroscopy to monitor electrode/electrolyte interfaces of lithium‐ion batteries under working conditions thus allowing relations between electrochemical performance and structural changes to be established." @default.
• W4226031763 created "2022-05-05" @default.
• W4226031763 creator A5018808535 @default.
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• W4226031763 date "2022-04-06" @default.
• W4226031763 modified "2023-10-14" @default.
• W4226031763 title "Monitoring electrode/electrolyte interfaces of Li‐ion batteries under working conditions: A surface‐enhanced Raman spectroscopic study on LiCoO₂ composite cathodes" @default.
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• W4226031763 doi "https://doi.org/10.1002/sia.7097" @default.
• W4226031763 hasPublicationYear "2022" @default.
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