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• W4226189957 abstract "Abstract Electrochemical conversion of CO 2 (CO 2 RR) has received significant attention since it could provide pathways for renewable energy storage to energy‐dense chemicals and synthetic fuels. We developed a novel CuO x /Cu/C type electrocatalyst via pyrolysis, which we used to convert CO 2 at industrially relevantly current densities using gas diffusion electrodes. The influence of the pyrolysis conditions on the electrocatalytic CO 2 RR activity and selectivity was evaluated. Optimization of the electrode structure to mitigate electrowetting was done by mixing the catalyst with polytetrafluoroethylene (PTFE). We found that mixing the most active catalyst with PTFE in a mass ratio of 1 to 0.25 substantially increased the formation of C 2 H 4 displaying 41% Faradaic efficiency (FE) at –240 mA cm –2 . Prolonged CO 2 RR at different current densities shows that the electrode containing 25 wt.% PTFE in the catalyst layer display FE C2H4 > 40% at –280 mA cm –2 for 2 h." @default.
• W4226189957 created "2022-05-05" @default.
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• W4226189957 date "2022-04-03" @default.
• W4226189957 modified "2023-10-14" @default.
• W4226189957 title "A CuO_x/Cu/C electrocatalyst‐based gas diffusion electrode for the electroreduction of CO₂ with high selectivity to C₂H₄" @default.
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• W4226189957 doi "https://doi.org/10.1002/elsa.202100200" @default.
• W4226189957 hasPublicationYear "2022" @default.
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