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- W4229000413 abstract "The fate of a Mott insulator under strong low frequency optical driving conditions is a fundamental problem in quantum many-body dynamics. Using ultrafast broadband optical spectroscopy, we measured the transient electronic structure and charge dynamics of an off-resonantly pumped Mott insulator Ca_{2}RuO_{4}. We observe coherent bandwidth renormalization and nonlinear doublon-holon pair production occurring in rapid succession within a sub-100-fs pump pulse duration. By sweeping the electric field amplitude, we demonstrate continuous bandwidth tuning and a Keldysh crossover from a multiphoton absorption to quantum tunneling dominated pair production regime. Our results provide a procedure to control coherent and nonlinear heating processes in Mott insulators, facilitating the discovery of novel out-of-equilibrium phenomena in strongly correlated systems." @default.
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- W4229000413 date "2022-05-06" @default.
- W4229000413 modified "2023-10-13" @default.
- W4229000413 title "Keldysh Space Control of Charge Dynamics in a Strongly Driven Mott Insulator" @default.
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- W4229000413 doi "https://doi.org/10.1103/physrevlett.128.187402" @default.
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