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• W4229017675 startingPage "410" @default.
• W4229017675 abstract "Ti3C2Tx has shown significant applications in many fields, such as electromagnetic interference (EMI) shielding and thermal camouflage. Yet, the preparation of high strength and functional Ti3C2Tx film is still challenging due to its weak interlayer interactions. Herein, we carefully design and synthesize a series of water-soluble polyacrylate polymers with different catechol group contents inspired by mussel byssus. Then, we assemble them with Ti3C2Tx by facile colloidal self-assembly approach, finally achieving robust and multifunctional Ti3C2Tx nanocomposite films through a nacre-mimetic construction strategy. These polymers combined with the Ti3C2Tx through hydrogen and coordination bonds, thus effectively enhancing the interfacial interactions of the nacre-mimetic films, resulting in the strength and toughness being enhanced to 4.5 and 4.4 times that of pure Ti3C2Tx film, respectively. Furthermore, the conductivities and EMI shielding efficiencies can be significantly improved by increasing the content of catechol groups in the polymers. Notably, we report for the first time that the ultrathin Ti3C2Tx nanocomposite films possess very low infrared emissivity (<0.2) and excellent infrared stealth performance, which can camouflage a high temperature surface of 100 °C to 33.8 °C. This biomimetic material design idea undoubtedly opens up a new path for constructing robust and multifunctional composite materials." @default.
• W4229017675 created "2022-05-08" @default.
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• W4229017675 date "2022-08-01" @default.
• W4229017675 modified "2023-09-29" @default.
• W4229017675 title "Robust biomimetic Ti3C2Tx nanocomposite films enhanced by mussel-inspired polymer for highly efficient electromagnetic shielding and thermal camouflage" @default.
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• W4229017675 doi "https://doi.org/10.1016/j.carbon.2022.05.004" @default.
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