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- W4229018863 abstract "Constructing photocatalysts with high activity and anti-photocorrosion is a key to harvesting hydrogen energy from seawater efficiently. Herein, graphene oxide closely coupled high-index facets CdZnS with rich sulfur vacancies (Vs-CZS@GO) has been successfully synthesized via one-pot sulfidation accompanied pyrolysis. DFT calculation confirmed the delicate surface/interface/defect engineering endowed high-index facets Vs-CZS@GO with a lower ΔGH* value and significant charge transfer behavior for efficient H2-generation. The synergistic effect of sulfur vacancy, high-index facets, and tightly coupling interface not only enhanced intrinsic active sites and carrier separation efficiencies, but also greatly promoted H2 evolution rate and stability. Consequently, Vs-CZS@GO displayed a significantly high H2-generation rate of 23.2 mmol∙g-1∙h-1 in natural seawater under visible-light irradiation, which is up to 82% of that in pure water. This work provides deeply insight into the synergistic regulation of electronic structure for exposed high-index facets photocatalysts via defect engineering and interface engineering for synergistic boosting visible-light-to-H2 evolution." @default.
- W4229018863 created "2022-05-08" @default.
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- W4229018863 date "2022-10-01" @default.
- W4229018863 modified "2023-10-18" @default.
- W4229018863 title "Graphene oxide coupled high-index facets CdZnS with rich sulfur vacancies for synergistic boosting visible-light-catalytic hydrogen evolution in natural seawater: Experimental and DFT study" @default.
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- W4229018863 doi "https://doi.org/10.1016/j.jcis.2022.05.008" @default.
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