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• W4229050023 startingPage "8327" @default.
• W4229050023 abstract "A novel photoanode was designed using the Cu–azolate framework (CuAF) and g-C3N4 as a core–shell nanocomposite (g-C3N4@CuAF) decorated with a Ni(OH)2 cocatalyst. The band structure of the g-C3N4@CuAF composite presented a heterojunction of staggered-gap type II. The transfer of photogenerated electrons and holes to relative low-energy bands of CuAF and g-C3N4 prevents their recombination so that the photocurrent density of g-C3N4@CuAF photoanode significantly increased compared to that of CuAF photoanode. The Ni(OH)2 cocatalyst loaded on the photoanodes provided a facile path for photogenerated holes to split water molecules. The photoconversion efficiency of the g-C3N4@CuAF/Ni(OH)2 photoanode was 6 times greater than that of the pristine CuAF. The photovoltage of 290 mV for the g-C3N4@CuAF/Ni(OH)2 photoanode compared to 189 mV for the CuAF/Ni(OH)2 photoanode indicates its deeper band bending. The g-C3N4@CuAF/Ni(OH)2 photoanode is stable under continuous light irradiation for 1 h." @default.
• W4229050023 created "2022-05-08" @default.
• W4229050023 creator A5060998998 @default.
• W4229050023 creator A5063547406 @default.
• W4229050023 creator A5063547608 @default.
• W4229050023 date "2022-05-05" @default.
• W4229050023 modified "2023-10-16" @default.
• W4229050023 title "Copper–Azolate Framework Coated on g-C₃N₄ Nanosheets as a Core–Shell Heterojunction and Decorated with a Ni(OH)₂ Cocatalyst for Efficient Photoelectrochemical Water Splitting" @default.
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• W4229050023 doi "https://doi.org/10.1021/acs.jpcc.2c01570" @default.
• W4229050023 hasPublicationYear "2022" @default.
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