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• W4229052170 abstract "Phase junctions of photocatalysts can promote the separation of photogenerated charge carriers for efficient utilization of the carriers. Construction of phase junctions and establishing their structure-performance relationship are still required. Herein, polycrystalline TiO2 decahedral plates with different phases were synthesized by thermal treatment-induced topotactic transition of titanium oxalate crystals. The phase of TiO2 evolved from pure anatase to anatase-brookite, anatase-brookite-rutile, and then to anatase-rutile, while the morphology of the decahedral plates was well maintained. The biphase anatase-brookite was found to be most efficient in photocatalytic hydrogen generation. Specifically, the hydrogen generation rate of the biphase anatase-brookite TiO2 was nearly 2.4 times greater than that of the biphase anatase-rutile TiO2. The spatially resolved surface photovoltage measurements indicate the more efficient separation of photogenerated charge carriers and thus greater photocatalytic activity of the former. This work provides a strategy for developing efficient phase-junction photocatalysts." @default.
• W4229052170 created "2022-05-08" @default.
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• W4229052170 date "2022-05-06" @default.
• W4229052170 modified "2023-10-18" @default.
• W4229052170 title "Constructing Anatase–Brookite TiO₂ Phase Junction by Thermal Topotactic Transition to Promote Charge Separation for Superior Photocatalytic H₂ Generation" @default.
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• W4229052170 doi "https://doi.org/10.1021/acs.jpclett.2c00964" @default.
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