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- W4229080691 abstract "One key challenge in photocatalytic hydrogen production is how to construct high-performance photocatalyst. Covalent triazine framework (CTF) based polymers as photocatalysts show great application potential because of their good photocatalytic activity, high chemical stability, tunable electronic and optical properties, and easy synthesis process. In this paper, we designed the ternary Z-scheme heterojunction [email protected]2-X%TrTh based on CTF polymer TrTh, TiO2 and Au nanoparticle, which exhibit higher photocatalytic hydrogen production rate compared with the corresponding binary heterojunction [email protected]2 and TiO2-12%TrTh. The results of photocatalytic hydrogen production show that the optimized [email protected]2-12%TrTh has a remarkable hydrogen production rate of 4288.54 μmol g−1 h−1, which is about 312.3 times of [email protected]2 and 9.1 times of the TiO2-12%TrTh. The enhanced hydrogen production activity of the ternary heterojunction comes from the local surface plasmonic resonance effect of Au nanoparticle, lower recombination efficiency of photogenerated electron-holes pairs and Z-scheme electron transfer pathway of [email protected]2-12%TrTh. The work provides a new strategy for designing efficient and practical photocatalyst." @default.
- W4229080691 created "2022-05-08" @default.
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- W4229080691 date "2022-05-01" @default.
- W4229080691 modified "2023-10-12" @default.
- W4229080691 title "Construction of ternary Z-scheme covalent triazine framework@Au@TiO2 for enhanced visible-light-driven hydrogen evolution activity" @default.
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- W4229080691 doi "https://doi.org/10.1016/j.ijhydene.2022.04.054" @default.
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