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- W4229368344 abstract "Contact prelithiation is an important strategy to compensate the initial capacity loss of lithium-ion batteries. However, the dead Li generated from inadequate Li conversion reduces the cycling stability of rechargeable batteries. Herein a mono-solvent dimethyl carbonate (DMC) electrolyte was employed in contact prelithiation for the first time. We discover that the low-organic-content raw electrolyte interphase (REI) induced by this electrolyte on Li source and anode is a mixed ion/electron conductor. Therefore, electron channels can be maintained even when the Li source has been completely wrapped by the DMC-derived REI. As a result, an outstanding Li source utilization of 92.8 % and a negligible dead Li yield can be realized. This strategy renders batteries with a very high initial Coulombic efficiency (90.0 %) and an excellent capacity retention (94.9 %) over 210 cycles, highlighting the significance of REI for effective contact prelithiation." @default.
- W4229368344 created "2022-05-10" @default.
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- W4229368344 date "2022-05-25" @default.
- W4229368344 modified "2023-10-16" @default.
- W4229368344 title "The Raw Mixed Conducting Interphase Affords Effective Prelithiation in Working Batteries" @default.
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- W4229368344 doi "https://doi.org/10.1002/anie.202205697" @default.
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