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• W4229661311 abstract "Abstract. Long-term ozone (O3) and nitric oxide (NOx) from fourteen state-of-the-art chemical transport models are evaluated and intercompared to ozone observations in East Asia, within the framework of the Model Inter-Comparison Study for ASIA phase III (MICS-ASIA III), designed to evaluate the capabilities and uncertainties of current chemical transport models (CTMs) simulations in Asia and provide multi-model estimates of pollution distributions. These models were run by fourteen independent groups in China, Japan, Korea, United States of America and other countries/regions. Compared with MICS-ASIAII, the evaluation against observations were extended to be one-full year in China and the western Pacific Rim from four months and the western Pacific Rim. Potential causes of the discrepancies between model results and observation have also been investigated by assessing the PBL heights, emission fluxes, dry deposition, O3-NOx relationships and vertical profiles among models in this study. In general, the model skills for O3 varied largely with region and seasons. Most models captured the key pattern of monthly and diurnal surface O3 and its precursors in North China Plain, Yangtze River Delta and western Pacific rim, but failed in Peral River Delta of China. A significant overestimation of surface ozone was found in May–September/October and January–May over North China Plain, western Pacific rim and Peral River Delta of China, respectively. A large intermodel variability of O3 existed in all subregions over East Asia in this study, which was caused by the internal parameterizations of chemistry, dry deposition and vertical mixing of models, even though the native schemes in models are similar. Ensemble average of 13 models on O3 did not always exhibit a superior performance compared to certain individual model, in contrast to its superiority in Europe. This suggested that the spread of ensemble-model values hadn't represented all uncertainties of ozone or most models in MICS-ASIAIII missed key processes. Compared with the previous phase of MICS-ASIA（MICS-ASIAII, this study improved the performance of ozone in March at Japan sites. But it predicted too enhanced surface O3 concentrations at western Japan in July, which has not been found in MICS-ASIAII. Major challenges still remain with regards to recognizing the sources of bias in surface O3 over East Asia in CTMs." @default.
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• W4229661311 date "2019-01-17" @default.
• W4229661311 modified "2023-09-25" @default.
• W4229661311 title "Model evaluation and inter-comparison of surface-level ozone and relevant species in East Asia in the context of MICS-Asia phase III Part I: overview" @default.
• W4229661311 doi "https://doi.org/10.5194/acp-2018-1283" @default.
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