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- W4230238105 abstract "Equations are derived for the d.c. current-voltage profile and the interfacial admittance of an electrode at which reactions occur according to the following scheme: O+ne⇄R⇄A⇵Y+ne⇄Z⇄B The assumption was made that the d.c. polarogram shows two well-separated waves, the first belonging to the reduction of O and the second to the reduction of both Y and O. The theory is based on a relatively simple diffusion-layer model of the d.c. processes occurring at the dropping mercury electrode, which appears to be a good approximation of the more complicated expanding sphere model. It is concluded that often the combination of d.c. polarographic data with the potential and frequency dependency of the interfacial admittance will lead to a satisfactory description of the electrode process." @default.
- W4230238105 created "2022-05-11" @default.
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- W4230238105 date "1973-06-25" @default.
- W4230238105 modified "2023-09-27" @default.
- W4230238105 title "A theoretical d.c. polarographic and faradaic impedance study of systems with first-order chemical reactions following and preceding the charge transfer step: the CEC and the CECEC mechanism" @default.
- W4230238105 doi "https://doi.org/10.1016/0368-1874(73)80138-8" @default.
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