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• W4230797257 abstract "The copper-catalyzed aerobic oxidation of primary and secondary alcohols without an external N-oxide co-oxidant is described. The catalyst system is composed of a Cu/diamine complex inspired by the enzyme tyrosinase, along with dimethylaminopyridine (DMAP) or N-methylimidazole (NMI). The Cu catalyst system works without 2,2,6,6-tetramethyl-l-piperidinoxyl (TEMPO) at ambient pressure and temperature, and displays activity for un-activated secondary alcohols, which remain a challenging substrate for catalytic aerobic systems. Our work underscores the importance of finding alternative mechanistic pathways for alcohol oxidation, which complement Cu/TEMPO systems, and demonstrate, in this case, a preference for the oxidation of activated secondary over primary alcohols." @default.
• W4230797257 created "2022-05-11" @default.
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• W4230797257 creator A5058300825 @default.
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• W4230797257 date "2015-02-10" @default.
• W4230797257 modified "2023-10-16" @default.
• W4230797257 title "A TEMPO-Free Copper-Catalyzed Aerobic Oxidation of Alcohols" @default.
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• W4230797257 doi "https://doi.org/10.1002/ange.201411483" @default.
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