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- W4232000558 abstract "Abstract Self‐assembled nanostructures of rod‐like molecules are commonly limited to nematic or layered smectic structures dominated by the parallel arrangement of the rod‐like components. Distinct self‐assembly behavior of four categories of dendritic rods constructed by placing a tri(hydroxy) group at the apex of dendritic oligo‐fluorenes is observed. Designed hydrogen bonding and dendritic architecture break the parallel arrangement of the rods, resulting in molecules with specific (fan‐like or cone‐like) shapes. While the fan‐shaped molecules tend to form hexagonal packing cylindrical phases, the cone‐shaped molecules could form spherical motifs to pack into various ordered structures, including the Frank–Kasper A15 phase and dodecagonal quasicrystal. This study provides a model system to engineer diverse supramolecular structures by rod‐like molecules and sheds new light into the mechanisms of the formation of unconventional spherical packing structures in soft matter." @default.
- W4232000558 created "2022-05-12" @default.
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- W4232000558 date "2019-07-17" @default.
- W4232000558 modified "2023-10-14" @default.
- W4232000558 title "Breaking Parallel Orientation of Rods via a Dendritic Architecture toward Diverse Supramolecular Structures" @default.
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- W4232000558 doi "https://doi.org/10.1002/ange.201904749" @default.
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