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- W4232351140 abstract "Abstract. We present the development of ANISORROPIA, the discrete adjoint of the ISORROPIA thermodynamic equilibrium model that treats the Na+-SO42−-HSO4−-NH4+-NO3−-Cl−-H2O aerosol system, and we demonstrate its sensitivity analysis capabilities. ANISORROPIA calculates sensitivities of an inorganic species in aerosol or gas phase with respect to the total concentrations of each species present with only a two-fold increase in computational time over the forward model execution. Due to the highly nonlinear and discontinuous solution surface of ISORROPIA, evaluation of the adjoint required a new, complex-variable version of the the model, which determines first-order sensitivities with machine precision and avoids cancellation errors arising from finite difference calculations. The adjoint is verified over an atmospherically relevant range of concentrations, temperature, and relative humidity. We apply ANISORROPIA to recent field campaign results from Atlanta, GA, USA, and Mexico City, Mexico, to characterize the inorganic aerosol sensitivities of these distinct urban air masses. The variability in the relationship between PM2.5 mass and precursor concentrations shown has important implications for air quality and climate. ANISORROPIA enables efficient elucidation of aerosol concentration dependence on aerosol precursor emissions in the context of atmospheric chemical transport model adjoints." @default.
- W4232351140 created "2022-05-12" @default.
- W4232351140 creator A5001150915 @default.
- W4232351140 creator A5036178078 @default.
- W4232351140 creator A5058462310 @default.
- W4232351140 creator A5067004889 @default.
- W4232351140 creator A5077420311 @default.
- W4232351140 date "2011-08-19" @default.
- W4232351140 modified "2023-09-27" @default.
- W4232351140 title "ANISORROPIA: the adjoint of the aerosol thermodynamic model ISORROPIA" @default.
- W4232351140 cites W1835577090 @default.
- W4232351140 cites W1964196637 @default.
- W4232351140 cites W1965687975 @default.
- W4232351140 cites W1966552855 @default.
- W4232351140 cites W1966774499 @default.
- W4232351140 cites W1967063733 @default.
- W4232351140 cites W1971290825 @default.
- W4232351140 cites W1974534908 @default.
- W4232351140 cites W1976817668 @default.
- W4232351140 cites W1977912107 @default.
- W4232351140 cites W1985498261 @default.
- W4232351140 cites W1987941491 @default.
- W4232351140 cites W1999866891 @default.
- W4232351140 cites W2001469987 @default.
- W4232351140 cites W2004184999 @default.
- W4232351140 cites W2004436064 @default.
- W4232351140 cites W2005812427 @default.
- W4232351140 cites W2006962396 @default.
- W4232351140 cites W2007715722 @default.
- W4232351140 cites W2008641894 @default.
- W4232351140 cites W2018673810 @default.
- W4232351140 cites W2019436394 @default.
- W4232351140 cites W2020876448 @default.
- W4232351140 cites W2026440788 @default.
- W4232351140 cites W2026923591 @default.
- W4232351140 cites W2028370128 @default.
- W4232351140 cites W2031803385 @default.
- W4232351140 cites W2035685316 @default.
- W4232351140 cites W2037357885 @default.
- W4232351140 cites W2037576794 @default.
- W4232351140 cites W2040291523 @default.
- W4232351140 cites W2040718868 @default.
- W4232351140 cites W2045576608 @default.
- W4232351140 cites W2046292519 @default.
- W4232351140 cites W2049766609 @default.
- W4232351140 cites W2049937033 @default.
- W4232351140 cites W2051375082 @default.
- W4232351140 cites W2056404295 @default.
- W4232351140 cites W2056447505 @default.
- W4232351140 cites W2057928955 @default.
- W4232351140 cites W2063474678 @default.
- W4232351140 cites W2065147121 @default.
- W4232351140 cites W2066743204 @default.
- W4232351140 cites W2074576826 @default.
- W4232351140 cites W2074662530 @default.
- W4232351140 cites W2074947155 @default.
- W4232351140 cites W2076112917 @default.
- W4232351140 cites W2078960528 @default.
- W4232351140 cites W2082745110 @default.
- W4232351140 cites W2095525251 @default.
- W4232351140 cites W2095939027 @default.
- W4232351140 cites W2096049379 @default.
- W4232351140 cites W2101506489 @default.
- W4232351140 cites W2110099732 @default.
- W4232351140 cites W2111369201 @default.
- W4232351140 cites W2116544321 @default.
- W4232351140 cites W2118141811 @default.
- W4232351140 cites W2121884510 @default.
- W4232351140 cites W2124684233 @default.
- W4232351140 cites W2124750468 @default.
- W4232351140 cites W2127093080 @default.
- W4232351140 cites W2131052934 @default.
- W4232351140 cites W2134134788 @default.
- W4232351140 cites W2136567789 @default.
- W4232351140 cites W2138017294 @default.
- W4232351140 cites W2138759632 @default.
- W4232351140 cites W2139197312 @default.
- W4232351140 cites W2143287674 @default.
- W4232351140 cites W2145411928 @default.
- W4232351140 cites W2146512399 @default.
- W4232351140 cites W2148278106 @default.
- W4232351140 cites W2148807170 @default.
- W4232351140 cites W2152181706 @default.
- W4232351140 cites W2153423813 @default.
- W4232351140 cites W2154564240 @default.
- W4232351140 cites W2158989459 @default.
- W4232351140 cites W2159722679 @default.
- W4232351140 cites W2161929247 @default.
- W4232351140 cites W2163741389 @default.
- W4232351140 cites W2164505281 @default.
- W4232351140 cites W2164687335 @default.
- W4232351140 cites W2164840653 @default.
- W4232351140 cites W2165449174 @default.
- W4232351140 cites W2165680013 @default.
- W4232351140 cites W2167968161 @default.
- W4232351140 cites W2168314263 @default.
- W4232351140 cites W2169769692 @default.
- W4232351140 cites W2170856910 @default.
- W4232351140 cites W2171812510 @default.
- W4232351140 cites W2605946006 @default.