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- W4233442807 abstract "Abstract Thionyl tetrafluoride (SOF 4 ) is a valuable connective gas for sulfur fluoride exchange (SuFEx) click chemistry that enables multidimensional linkages to be created via sulfur–oxygen and sulfur–nitrogen bonds. Herein, we expand the available SuFEx chemistry of SOF 4 to include organolithium nucleophiles, and demonstrate, for the first time, the controlled projection of sulfur–carbon links at the sulfur center of SOF 4 ‐derived iminosulfur oxydifluorides (R 1 −N=SOF 2 ). This method provides rapid and modular access to sulfonimidoyl fluorides (R 1 −N=SOFR 2 ), another array of versatile SuFEx connectors with readily tunable reactivity of the S−F handle. Divergent connections derived from these valuable sulfonimidoyl fluoride units are also demonstrated, including the synthesis of sulfoximines, sulfonimidamides, and sulfonimidates." @default.
- W4233442807 created "2022-05-12" @default.
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- W4233442807 date "2018-01-16" @default.
- W4233442807 modified "2023-10-16" @default.
- W4233442807 title "SuFEx Chemistry of Thionyl Tetrafluoride (SOF<sub>4</sub> ) with Organolithium Nucleophiles: Synthesis of Sulfonimidoyl Fluorides, Sulfoximines, Sulfonimidamides, and Sulfonimidates" @default.
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- W4233442807 doi "https://doi.org/10.1002/ange.201712145" @default.
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