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• W4234011536 abstract "The bis(imino)pyridine 2,6-(2,6-iPr2-C6H3NCPh)2-C5H3N (iPrBPDI) molybdenum dinitrogen complex, [{(iPrBPDI)Mo(N2)}2(μ2,η1,η1-N2)] has been prepared and contains both weakly (terminal) and modestly (bridging) activated N2 ligands. Addition of ammonia resulted in sequential NH bond activations, thus forming bridging parent imido (μ-NH) ligands with concomitant reduction of one of the imines of the supporting chelate. Using primary and secondary amines, model intermediates have been isolated that highlight the role of metal–ligand cooperativity in NH3 oxidation." @default.
• W4234011536 created "2022-05-12" @default.
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• W4234011536 date "2014-10-16" @default.
• W4234011536 modified "2023-10-16" @default.
• W4234011536 title "Synthesis and Ligand Modification Chemistry of a Molybdenum Dinitrogen Complex: Redox and Chemical Activity of a Bis(imino)pyridine Ligand" @default.
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• W4234011536 doi "https://doi.org/10.1002/ange.201408725" @default.
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