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- W4235087888 abstract "Abstract (−)‐Daphnilongeranin B and (−)‐daphenylline are two hexacyclic Daphniphyllum alkaloids, each containing a complex cagelike backbone. Described herein are the first asymmetric total synthesis of (−)‐daphnilongeranin B and a bioinspired synthesis of (−)‐daphenylline with an unusual E ring embedded in a cagelike framework. The key features include an intermolecular [3+2] cycloaddition, a late‐stage aldol cyclization to install the F ring of daphnilongeranin B, and a bioinspired cationic rearrangement leading to the tetrasubstituted benzene ring of daphenylline." @default.
- W4235087888 created "2022-05-12" @default.
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- W4235087888 date "2017-12-05" @default.
- W4235087888 modified "2023-10-17" @default.
- W4235087888 title "Divergent Total Syntheses of (−)‐Daphnilongeranin B and (−)‐Daphenylline" @default.
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- W4235087888 doi "https://doi.org/10.1002/ange.201709762" @default.
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