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- W4236064320 abstract "Abstract An efficient metal‐free cascade reaction between 1‐dibromovinyl‐2‐nitro‐substituted arenes and secondary amines results in the formation of polycyclic pseudoindoxyls in a single step. The reaction mechanism leading to these fused ring systems was investigated, and is believed to involve the initial formation of nitroarylated ynamines/ynamides. These intermediates cycloisomerize towards N‐alkenyl‐tethered 2‐aminoisatogens via a carbene intermediate as demonstrated by QTAIM (quantum theory of atoms in molecules) and ELF (electron localization function) analysis. A subsequent intramolecular dipolar cycloaddition afforded the title compounds." @default.
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- W4236064320 date "2018-04-16" @default.
- W4236064320 modified "2023-09-26" @default.
- W4236064320 title "Metal-Free Cyclization of <i>ortho</i> -Nitroaryl Ynamides and Ynamines towards Spiropseudoindoxyls" @default.
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- W4236064320 doi "https://doi.org/10.1002/ange.201800340" @default.
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