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- W4236693110 abstract "Multiphoton dissociation/ionisation studies have been carried out at 355 nm for dimethyl disulfide (CH3SSCH3) using a time-of-flight-mass spectrometer. The prominent ion signals observed are CH3+, S+, HCS+ and S2+. No evidence for the formation of a parent ion signal was observed. The laser power variation experiments show a two-photon dependence for the most prominent HCS+ ion. The presence of a signal at m/e 30 is explained in terms of concerted elimination of ethane from the excited neutral CH3SSCH3 via a cyclic transition state. It is inferred that the multiphoton dissociation of CH3SSCH3 at 355 nm involves both S-S and C-S bond cleavage. Based on these results, it has been suggested that CH3S+ isomerises to CH2SH+, which undergoes unimolecular decay to produce HCS+ by H2 elimination. The results have been interpreted in terms of the dissociation of the parent molecule using two photons, followed by the ionisation of the fragments. Copyright © 2001 John Wiley & Sons, Ltd." @default.
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- W4236693110 date "2001-10-30" @default.
- W4236693110 modified "2023-09-27" @default.
- W4236693110 title "Multiphoton dissociation/ionisation of dimethyl sulfide" @default.
- W4236693110 doi "https://doi.org/10.1002/rcm.464.abs" @default.
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