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- W4237544742 abstract "Abstract The kinetic lability of hexadentate gallium‐based tripods is sufficient to ensure thermodynamic self‐assembly of luminescent heterodimetallic [GaLn( L3 ) 3 ] 6+ helicates on the hour time scale, where Ln is a trivalent 4f‐block cation. The inertness is, however, large enough for preserving the triple‐helical structure when [GaLn( L3 ) 3 ] 6+ is exposed to lanthanide exchange. The connection of a second gallium‐based tripod further slows down the exchange processes to such an extent that spectroscopically active [CrErCr( L4 ) 3 ] 9+ can be diluted into closed‐shell [GaYGa( L4 ) 3 ] 9+ matrices without metal scrambling. This feature is exploited for pushing molecular‐based energy‐transfer upconversion (ETU) at room temperature." @default.
- W4237544742 created "2022-05-12" @default.
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- W4237544742 date "2017-10-16" @default.
- W4237544742 modified "2023-09-25" @default.
- W4237544742 title "Controlling Lanthanide Exchange in Triple-Stranded Helicates: A Way to Optimize Molecular Light-Upconversion" @default.
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- W4237544742 doi "https://doi.org/10.1002/ange.201709156" @default.
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