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• W4238049494 startingPage "917" @default.
• W4238049494 abstract "A recently proposed procedure for computing the S matrix for collinear molecular collisions is extended from the single-mode case to the multimode case. In this procedure the semiclassical Hamiltonian describing the molecular collision is integrated in a finite-dimensional, faithful nonunitary representation of the dynamical group. When the integration is completed, the resulting group operation is mapped into the infinite-dimensional unitary representation to describe the S matrix which acts on the molecular Hilbert space and describes collisional excitation of the internal vibrational modes. This procedure is implemented to study the two-mode collision process N2+O2 and the two three-mode collision processes N2+CO2 and NO+CO2. The results compare favorably with other treatments of these collinear collision processes." @default.
• W4238049494 created "2022-05-12" @default.
• W4238049494 creator A5040578695 @default.
• W4238049494 creator A5081258957 @default.
• W4238049494 date "1989-07-15" @default.
• W4238049494 modified "2023-09-27" @default.
• W4238049494 title "Group theoretical approach to semiclassical dynamics: Multimode case" @default.
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• W4238049494 doi "https://doi.org/10.1063/1.457142" @default.
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