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- W4238059735 abstract "A highly stereoselective route to functionalized pyrrolidines by the metal-catalyzed diverted N−H insertion of a range of diazocarbonyl compounds with β-aminoketone derivatives is described. A number of catalysts (rhodium(II) carboxylate dimers, copper(I) triflate, and an iron(III) porphyrin) are shown to promote the process under mild conditions to give a wide range of highly substituted proline derivatives. The reaction starts as a metallocarbene N−H insertion but is diverted by an intermolecular aldol reaction." @default.
- W4238059735 created "2022-05-12" @default.
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- W4238059735 date "2016-02-05" @default.
- W4238059735 modified "2023-09-25" @default.
- W4238059735 title "Stereoselective Synthesis of Functionalized Pyrrolidines by the Diverted N−H Insertion Reaction of Metallocarbenes with β-Aminoketone Derivatives" @default.
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- W4238059735 doi "https://doi.org/10.1002/ange.201511433" @default.
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