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• W4238076575 endingPage "23590" @default.
• W4238076575 startingPage "23582" @default.
• W4238076575 abstract "Electrocatalytic reduction of CO2 by metal–organic frameworks (MOFs) has been widely investigated, but insufficient conductivity limits application. Herein, a porous 3D In-MOF {(Me2NH2)[In(BCP)]⋅2 DMF}n (V11) with good stability was constructed with two types of channels (1.6 and 1.2 nm diameter). V11 exhibits moderate catalytic activity in CO2 electroreduction with 76.0 % of Faradaic efficiency for formate (FEHCOO-). Methylene blue molecules of suitable size and pyrolysis temperature were introduced and transformed into carbon particles (CPs) after calcination. The performance of the obtained CPs@V11 is significantly improved both in FEHCOO- (from 76.0 % to 90.1 %) and current density (2.2 times). Control experiments show that introduced CPs serve as accelerant to promote the charges and mass transfer in framework, and benefit to sufficiently expose active sites. This strategy can also work on other In-MOFs, demonstrating the universality of this method for electroreduction of CO2." @default.
• W4238076575 created "2022-05-12" @default.
• W4238076575 creator A5015559567 @default.
• W4238076575 creator A5046881277 @default.
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• W4238076575 creator A5074202565 @default.
• W4238076575 creator A5077660409 @default.
• W4238076575 creator A5088006335 @default.
• W4238076575 date "2021-09-13" @default.
• W4238076575 modified "2023-10-03" @default.
• W4238076575 title "A Facile Strategy for Constructing a Carbon‐Particle‐Modified Metal–Organic Framework for Enhancing the Efficiency of CO ₂ Electroreduction into Formate" @default.
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