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- W4238433033 abstract "Abstract A new class of stabilized pentacene derivatives with externally fused five‐membered rings are prepared by means of a key palladium‐catalyzed cyclopentannulation step. The target compounds are synthesized by chemical manipulation of a partially saturated 6,13‐dibromopentacene precursor that can be fully aromatized in a final step through a DDQ‐mediated dehydrogenation reaction (DDQ=2,3‐dichloro‐5,6‐dicyano‐1,4‐benzoquinone). The new 1,2,8,9‐tetraaryldicyclopenta[fg,qr]pentacene derivatives have narrow energy gaps of circa 1.2 eV and behave as strong electron acceptors with lowest unoccupied molecular orbital energies between −3.81 and −3.90 eV. Photodegradation studies reveal the new compounds are more photostable than 6,13‐bis(triisopropylsilylethynyl)pentacene (TIPS‐pentacene)." @default.
- W4238433033 created "2022-05-12" @default.
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- W4238433033 date "2015-11-19" @default.
- W4238433033 modified "2023-09-30" @default.
- W4238433033 title "Stabilizing Pentacene By Cyclopentannulation" @default.
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- W4238433033 doi "https://doi.org/10.1002/ange.201508650" @default.
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