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• W4239121921 startingPage "16057" @default.
• W4239121921 abstract "Abstract Aprocess for the assembly of carbazole alkaloids has been developed on the basis of ring‐closing metathesis (RCM) and ringrearrangement–aromatization (RRA) as the key steps. This method is based on allyl Grignard addition to isatin derivatives to provide smooth access to 2,2‐diallyl 3‐oxindole derivatives through a 1,2‐allyl shift. The diallyl derivatives were used as RCM precursors to afford a novel class of spirocyclopentene‐3‐oxindole derivatives, which underwent a novel RRA reaction to afford carbazole derivatives. The synthetic sequence to carbazoles was shortened by combining the RCM and RRA steps in an orthogonal tandem catalytic process. The utility of this methodology was further demonstrated by the straightforward synthesis of carbazole alkaloids, including amukonal derivative, girinimbilol, heptaphylline, and bis(2‐hydroxy‐3‐methylcarbazole)." @default.
• W4239121921 created "2022-05-12" @default.
• W4239121921 creator A5005828640 @default.
• W4239121921 creator A5025861277 @default.
• W4239121921 creator A5044571294 @default.
• W4239121921 creator A5091537274 @default.
• W4239121921 date "2015-11-19" @default.
• W4239121921 modified "2023-10-18" @default.
• W4239121921 title "Synthesis of Carbazole Alkaloids by Ring‐Closing Metathesis and Ring Rearrangement–Aromatization" @default.
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• W4239121921 doi "https://doi.org/10.1002/ange.201508746" @default.
• W4239121921 hasPublicationYear "2015" @default.
• W4239121921 type Work @default.
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