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• W4239392014 abstract "Abstract Substitution of a histidine, comprising part of the catalytic base group in the ent‐copalyl diphosphate synthases found in all seed plants for gibberellin phytohormone metabolism, by a larger aromatic residue leads to rearrangements. Through a series of 1,2‐hydride and methyl shifts of the initially formed bicycle predominant formation of (−)‐kolavenyl diphosphate is observed. Further mutational analysis and quantum chemical calculations provide mechanistic insight into the basis for this profound effect on product outcome." @default.
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• W4239392014 date "2015-11-25" @default.
• W4239392014 modified "2023-10-07" @default.
• W4239392014 title "Blocking Deprotonation with Retention of Aromaticity in a Plant <i>ent</i> -Copalyl Diphosphate Synthase Leads to Product Rearrangement" @default.
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• W4239392014 doi "https://doi.org/10.1002/ange.201509060" @default.
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