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- W4239510694 abstract "Design of green, safe, and sustainable process for the synthesis of hydrogen peroxide (H2O2) is a very important subject. Early reported processes, however, require hydrogen (H2) and palladium-based catalysts. Herein we propose a photocatalytic process for H2O2 synthesis driven by metal-free catalysts with earth-abundant water and molecular oxygen (O2) as resources under sunlight irradiation (λ>400 nm). We use graphitic carbon nitride (g-C3N4) containing electron-deficient aromatic diimide units as catalysts. Incorporating the diimide units positively shifts the valence-band potential of the catalysts, while maintaining sufficient conduction-band potential for O2 reduction. Visible light irradiation of the catalysts in pure water with O2 successfully produces H2O2 by oxidation of water by the photoformed valence-band holes and selective two-electron reduction of O2 by the conduction band electrons." @default.
- W4239510694 created "2022-05-12" @default.
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- W4239510694 date "2014-10-07" @default.
- W4239510694 modified "2023-10-18" @default.
- W4239510694 title "Sunlight-Driven Hydrogen Peroxide Production from Water and Molecular Oxygen by Metal-Free Photocatalysts" @default.
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- W4239510694 doi "https://doi.org/10.1002/ange.201407938" @default.
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