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- W4239947348 abstract "A strategy to covalently connect crystalline covalent organic frameworks (COFs) with semiconductors to create stable organic–inorganic Z-scheme heterojunctions for artificial photosynthesis is presented. A series of COF–semiconductor Z-scheme photocatalysts combining water-oxidation semiconductors (TiO2, Bi2WO6, and α-Fe2O3) with CO2 reduction COFs (COF-316/318) was synthesized and exhibited high photocatalytic CO2-to-CO conversion efficiencies (up to 69.67 μmol g−1 h−1), with H2O as the electron donor in the gas–solid CO2 reduction, without additional photosensitizers and sacrificial agents. This is the first report of covalently bonded COF/inorganic-semiconductor systems utilizing the Z-scheme applied for artificial photosynthesis. Experiments and calculations confirmed efficient semiconductor-to-COF electron transfer by covalent coupling, resulting in electron accumulation in the cyano/pyridine moieties of the COF for CO2 reduction and holes in the semiconductor for H2O oxidation, thus mimicking natural photosynthesis." @default.
- W4239947348 created "2022-05-12" @default.
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- W4239947348 date "2020-02-25" @default.
- W4239947348 modified "2023-10-15" @default.
- W4239947348 title "Semiconductor/Covalent‐Organic‐Framework Z‐Scheme Heterojunctions for Artificial Photosynthesis" @default.
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- W4239947348 doi "https://doi.org/10.1002/ange.202000929" @default.
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