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- W4240177046 abstract "Abstract Treatment of alkenylstannanes with Cu(OAc) 2 /Et 3 N affords the corresponding enol esters or ketones under conditions that proved compatible with many common functionalities; these include groups that would neither survive under the standard Tamao–Fleming conditions for the oxidation of C −SiR 3 bonds nor under the conditions commonly used to oxidize C−B bonds. Chiral centers adjacent to the unveiled carbonyls are not racemized and competing protodestannation is marginal, even if the substrate carries unprotected −OH groups as internal proton sources. Therefore, the procedure is well suited for the preparation of acyloin and aldol derivatives. These enabling virtues are illustrated by a concise approach to the bicyclic lipid paecilonic acid A." @default.
- W4240177046 created "2022-05-12" @default.
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- W4240177046 date "2017-04-21" @default.
- W4240177046 modified "2023-10-01" @default.
- W4240177046 title "A Method for the Late‐Stage Formation of Ketones, Acyloins, and Aldols from Alkenylstannanes: Application to the Total Synthesis of Paecilonic Acid A" @default.
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- W4240177046 doi "https://doi.org/10.1002/ange.201701391" @default.
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