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• W4240217008 abstract "Abstract The Friedel–Crafts acylation is commonly used for the synthesis of aryl ketones, and a biocatalytic version, which may benefit from the chemo‐ and regioselectivity of enzymes, has not yet been introduced. Described here is a bacterial acyltransferase which can catalyze Friedel–Crafts C‐acylation of phenolic substrates in buffer without the need of CoA‐activated reagents. Conversions reach up to >99 %, and various C‐ or O‐acyl donors, such as DAPG or isopropenyl acetate, are accepted by this enzyme. Furthermore the enzyme enables a Fries rearrangement‐like reaction of resorcinol derivatives. These findings open an avenue for the development of alternative and selective C−C bond formation methods." @default.
• W4240217008 created "2022-05-12" @default.
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• W4240217008 date "2017-05-23" @default.
• W4240217008 modified "2023-10-16" @default.
• W4240217008 title "Biocatalytic Friedel–Crafts Acylation and Fries Reaction" @default.
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• W4240217008 doi "https://doi.org/10.1002/ange.201703270" @default.
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