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- W4240614239 abstract "The construction of a spatially defined assembly of molecular building blocks, especially in the vertical direction, presents a great challenge for surface molecular engineering. Herein, we demonstrate that an electric field applied between an STM tip and a substrate triggered the formation of a bilayer structure at the solid–liquid interface. In contrast to the typical high electric-field strength (109 V m−1) used to induce structural transitions in supramolecular assemblies, a mild electric field (105 V m−1) triggered the formation of a bilayer structure of a polar molecule on top of a nanoporous network of trimesic acid on graphite. The bilayer structure was transformed into a monolayer kagome structure by changing the polarity of the electric field. This tailored formation and large-scale phase transformation of a molecular assembly in the perpendicular dimension by a mild electric field opens perspectives for the manipulation of surface molecular nanoarchitectures." @default.
- W4240614239 created "2022-05-12" @default.
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- W4240614239 date "2014-11-06" @default.
- W4240614239 modified "2023-10-17" @default.
- W4240614239 title "Bilayer Molecular Assembly at a Solid/Liquid Interface as Triggered by a Mild Electric Field" @default.
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- W4240614239 doi "https://doi.org/10.1002/ange.201406523" @default.
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