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- W4241189303 abstract "Abstract The garnet electrolyte presents poor wettability with Li metal, resulting in an extremely large interfacial impedance and drastic growth of Li dendrites. Herein, a novel ultra‐stable conductive composite interface (CCI) consisting of Li y Sn alloy and Li 3 N is constructed in situ between Li 6.4 La 3 Zr 1.4 Ta 0.6 O 12 (LLZTO) pellet and Li metal by a conversion reaction of SnN x with Li metal at 300 °C. The Li y Sn alloy as a continuous and robust bridge between LLZTO and Li metal can effectively reduce the LLZTO/Li interfacial resistance from 4468.0 Ω to 164.8 Ω. Meanwhile, the Li 3 N as a fast Li‐ion channel can efficiently transfer Li ions and give their uniform distribution at the LLZTO/Li interface. Therefore, the Li/LLZTO@CCI/Li symmetric battery stably cycles for 1200 h without short circuit, and the all‐solid‐state high‐voltage Li/LLZTO@CCI/LiNi 0.5 Co 0.2 Mn 0.3 O 2 battery achieves a specific capacity of 161.4 mAh g −1 at 0.25 C with a capacity retention rate of 92.6 % and coulombic efficiency of 100.0 % after 200 cycles at 25 °C." @default.
- W4241189303 created "2022-05-12" @default.
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- W4241189303 date "2020-06-02" @default.
- W4241189303 modified "2023-10-12" @default.
- W4241189303 title "In Situ Construction of an Ultra‐Stable Conductive Composite Interface for High‐Voltage All‐Solid‐State Lithium Metal Batteries" @default.
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- W4241189303 doi "https://doi.org/10.1002/ange.202000547" @default.
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