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- W4241275285 abstract "The heterometallic complexes trans-[Cp(dppe)FeNCRu(o-bpy)CNFe(dppe)Cp][PF6]n (1[PF6]n, n=2, 3, 4; o-bpy=1,2-bis(2,2′-bipyridyl-6-yl)ethane, dppe=1,2-bis(diphenylphosphino)ethane, Cp=1,3-cyclopentadiene) in three distinct states have been synthesized and fully characterized. 13+[PF6]3 and 14+[PF6]4 are the one- and two-electron oxidation products of 12+[PF6]2, respectively. The investigated results suggest that 1[PF6]3 is a Class II mixed valence compound. 1[PF6]4 after a thermal treatment at 400 K shows an unusually delocalized mixed valence state of [FeIII-NC-RuIII-CN-FeII], which is induced by electron transfer from the central RuII to the terminal FeIII in 1[PF6]4, which was confirmed by IR spectroscopy, magnetic data, and EPR and Mössbauer spectroscopy." @default.
- W4241275285 created "2022-05-12" @default.
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- W4241275285 date "2017-01-12" @default.
- W4241275285 modified "2023-09-23" @default.
- W4241275285 title "An Unusually Delocalized Mixed-Valence State of a Cyanidometal-Bridged Compound Induced by Thermal Electron Transfer" @default.
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- W4241275285 doi "https://doi.org/10.1002/ange.201610855" @default.
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