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- W4241281465 abstract "Colloidal crystallization can be programmed using building blocks consisting of a nanoparticle core and DNA bonds to form materials with controlled crystal symmetry, lattice parameters, stoichiometry, and dimensionality. In the context of DNA-mediated nanoparticle crystallization, the most stable interactions often contain the greatest number of hybridization events, or “bonding” interactions, between the DNA ligands on neighboring particles. The relative ratio between surface area and D necessary to observe equilibrium habits likely reflects the hydrodynamic truncation where the geometric and DNA driving forces both favor body-centered cubic symmetry. Importantly, the face-to-face interactions that occur within this zone of anisotropy possess greater fractions of hybridized DNA and greater rotational restrictions than spherical nanoparticles, which in principle, should enable experimental realization of equilibrium habits. Facet yield captures how favorable the growth conditions are for the expected facet, while the habit yield additionally factors in nucleation and sample preparation effects." @default.
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- W4241281465 date "2020-08-31" @default.
- W4241281465 modified "2023-10-16" @default.
- W4241281465 title "Programming Colloidal Crystal Habit with Anisotropic Nanoparticle Building Blocks and DNA Bonds*" @default.
- W4241281465 doi "https://doi.org/10.4324/9780429200151-33" @default.
- W4241281465 hasPublicationYear "2020" @default.
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